CobaltMaghrebV1, France, Analysis, bibRecord, 000211

On the mechanism of the P2-Na0.70CoO2→O2-LiCoO2 exchange reaction. Part I: proposition of a model to describe the P2-02 transition

Identifieur interne : 000211 ( France/Analysis ); précédent : 000210; suivant : 000212

On the mechanism of the P2-Na0.70CoO2→O2-LiCoO2 exchange reaction. Part I: proposition of a model to describe the P2-02 transition

Auteurs : F. Tournadre [France] ; L. Croguennec [France] ; I. Saadoune [France, Maroc] ; D. Carlier [France] ; Y. Shoe-Horn [France] ; P. Willmann [France] ; C. Delmas [France]

Source :

Journal of solid state chemistry : (Print) [ 0022-4596 ] ; 2004.

RBID : Pascal:05-0019356

Descripteurs français

Pascal (Inist)
- Etude expérimentale, Interaction échange, Nucléation, Défaut empilement, Simulation numérique, Diffraction RX, Sodium oxyde, Cobalt oxyde, Composé ternaire, Lithium oxyde, Structure lamellaire, Na0,70CoO2, Co Na O, LiCoO2, Co Li O, 6460Q, 6172N.

English descriptors

KwdEn :
- Cobalt oxides, Digital simulation, Exchange interactions, Experimental study, Lamellar structure, Lithium oxides, Nucleation, Sodium oxides, Stacking faults, Ternary compounds, XRD.

Abstract

A model was proposed to describe the exchange reaction of sodium by lithium in P2 crystals. The exchange consists on the formation of nucleation centers and then on the growth of O2 domains in P2 crystals from these nucleation centers. Octahedral environments for lithium ions are obtained when one slab over two glides by (2/3,1/3,0) or by (1/3,2/3,0) in P2 structure. The existence of two different gliding vectors should lead to stacking faulted structures that can be simulated using DIFFaX software. The comparison of simulated and experimental XRD patterns for 02- LiCoO₂(ex-Na_0.7CoO₂) has shown that in that case the growth of the O2 domains in the P2 crystals is faster than the formation of nucleation centers.

Affiliations:

Links toward previous steps (curation, corpus...)

to stream PascalFrancis, to step Corpus: 000203
to stream PascalFrancis, to step Curation: 000092
to stream PascalFrancis, to step Checkpoint: 000201
to stream Main, to step Merge: 000A15
to stream Main, to step Curation: 000A02
to stream Main, to step Exploration: 000A02
to stream France, to step Extraction: 000211

Links to Exploration step

Pascal:05-0019356

Le document en format XML

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 exchange reaction. Part I: proposition of a model to describe the P2-02 transition</title>
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 exchange reaction. Part I: proposition of a model to describe the P2-02 transition</title>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Cobalt oxides</term>
<term>Digital simulation</term>
<term>Exchange interactions</term>
<term>Experimental study</term>
<term>Lamellar structure</term>
<term>Lithium oxides</term>
<term>Nucleation</term>
<term>Sodium oxides</term>
<term>Stacking faults</term>
<term>Ternary compounds</term>
<term>XRD</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Etude expérimentale</term>
<term>Interaction échange</term>
<term>Nucléation</term>
<term>Défaut empilement</term>
<term>Simulation numérique</term>
<term>Diffraction RX</term>
<term>Sodium oxyde</term>
<term>Cobalt oxyde</term>
<term>Composé ternaire</term>
<term>Lithium oxyde</term>
<term>Structure lamellaire</term>
<term>Na0,70CoO2</term>
<term>Co Na O</term>
<term>LiCoO2</term>
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<front><div type="abstract" xml:lang="en">A model was proposed to describe the exchange reaction of sodium by lithium in P2 crystals. The exchange consists on the formation of nucleation centers and then on the growth of O2 domains in P2 crystals from these nucleation centers. Octahedral environments for lithium ions are obtained when one slab over two glides by (2/3,1/3,0) or by (1/3,2/3,0) in P2 structure. The existence of two different gliding vectors should lead to stacking faulted structures that can be simulated using DIFFaX software. The comparison of simulated and experimental XRD patterns for 02- LiCoO<sub>2</sub>
(ex-Na<sub>0.7</sub>
CoO<sub>2</sub>
) has shown that in that case the growth of the O2 domains in the P2 crystals is faster than the formation of nucleation centers.</div>
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	Serveur d'exploration sur le cobalt au Maghreb
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Serveur d'exploration sur le cobalt au Maghreb

On the mechanism of the P2-Na0.70CoO2→O2-LiCoO2 exchange reaction. Part I: proposition of a model to describe the P2-02 transition

On the mechanism of the P2-Na0.70CoO2→O2-LiCoO2 exchange reaction. Part I: proposition of a model to describe the P2-02 transition

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